World record attosecond measurement at SwissFEL

As scientists push X-ray free electron lasers into the attosecond regime, diagnostic tools with higher precision are needed. Now scientists at the Paul Scherrer Institute PSI have demonstrated the ability to characterise pulses as short as 300 attoseconds: a world record time-resolution using electron-beam streaking.

X-ray free electron lasers such as SwissFEL generate short and powerful pulses of X-ray light that allow scientists to study atomic and molecular processes in action. Scientists are now striving to generate shorter and shorter pulses to access attosecond timescales (10-18 s) and observe the motion of electrons in real time.

Capturing such ultrafast processes with X-rays requires not only attosecond pulses; it also requires ways to precisely characterise the X-rays. “You need to know exactly how long each pulse lasts for and when the brightest parts of the pulse hit, for example,” says Eduard Prat, scientist in the beam dynamics group at SwissFEL. “For many scientific applications, if you don’t have this information, you’re blind.” 

A team from PSI has recently demonstrated that the PolariX – a type of radiofrequency deflector device developed by PSI in collaboration with CERN and the German research centre DESY – can meet the ambitious requirements of attosecond science. 

The electrons tell the story of the X-rays they made.

To create the X-ray light in the SwissFEL, bunches of electrons are accelerated to close to the speed of light and wiggled in a series of magnets called undulators, whereby they emit intense bursts of photons – the X-ray pulses. 

At attosecond timescales, it’s difficult to measure the properties of these pulse directly in a reliable way. X-rays interact only weakly with matter, and traditional sensors aren’t fast enough to resolve attosecond-scale events. Instead, scientists can study the electrons that produced them. 

Sitting after the undulators, the PolariX measures the electron bunch after they’ve released their photons. The device bends the beam using a radiofrequency field, spreading out the electrons depending on their exact arrival time – a method known as electron beam streaking. From the spread, the length of each individual electron bunch can be measured.

When the electrons emit photons (in technical terms, they ‘lase’), they lose energy. By measuring this energy difference, and how it is spread at the parts of the electron beam that lase, PolariX provides information on the X-ray pulse, in particular how its intensity varies over time.

A #MadeAtPSI success story

Although electron streaking is a relatively well-established technique for X-ray pulse characterisation, what makes PolariX unusual is that it can streak in any direction, helping to fully characterise the electron bunch – a concept invented at CERN and realised thanks to the radiofrequency technology at PSI. In contrast, most other devices only streak in one direction, giving limited information about the electron beam. 

During the last seven years of development at PSI, the PolariX has become one of the world leading devices for this purpose. Five devices are in operation at DESY in Germany, with whom the device was developed, and the team at PSI is currently in discussion with other institutes worldwide to provide them with their RF technologies.

“Pretty much all of the systems and components of PolariX were made at PSI,” says Paolo Craievich, who leads the RF systems group at PSI. “Over the course of PolariX’s development, we have become very experienced, and now we are leading in the world. I’m very proud for the whole RF section – it’s the work from many different people.” 

Read more on PSI website

Image: Eduard Prat (left) and Paolo Craievich in SwissFEL – proud of the teamwork that has now led to a world record time-resolution in X-ray pulse measurement using electron-beam streaking. © Paul Scherrer Institute PSI/Mahir Dzambegovic

Credit: Paul Scherrer Institute PSI/Mahir Dzambegovic

SwissFEL: a next generation tool for Attosecond Science

The 2023 Nobel Prize in Physics was awarded for the development of attosecond science – a field that sheds light on the movement of electrons on their natural timescale. Several researchers at the Swiss X-ray free electron laser SwissFEL are recognised in the scientific background to this prize. This is no coincidence. With recent technical developments enabling attosecond and fully coherent X-ray pulses, SwissFEL promises to rapidly advance this emerging research area.

“We can now open the door to the world of electrons. Attosecond physics gives us the opportunity to understand mechanisms that are governed by electrons. The next step will be utilising them.” So said Eva Olsson, Chair of the Nobel Committee for Physics at the Royal Swedish Academy of Sciences, at the announcement of the 2023 Nobel Prize in Physics.

The prize was awarded to Pierre Agostini, Ferenc Krausz and Anne L’Huillier “for experimental methods that generate attosecond pulses of light for the study of electron dynamics in matter”. These breakthrough experimental methods are based on table-top laser systems – that is, laser systems that roughly fit onto an optical table and generate light mainly in the extreme ultraviolet energy range. Yet, in order to truly utilise our new insight into the world of electrons, further technological advances will be important that probe the movements of electrons in a wide variety of functional materials.

The scientific background produced by the Royal Swedish Academy of Sciences recognises the contributions from several researchers at PSI. There is a unifying theme to these researchers: they all now work at SwissFEL on upgrades that are enabling attosecond X-ray pulses, combining the possibilities of this astounding time resolution with the higher photon energies and higher photon fluxes offered by free electron laser light.

The contributions of these PSI researchers all lay in making the first steps of extending attosecond techniques, first developed in the gas phase, to new phases of matter – liquids and solids.

Read more on PSI website

Image: Contributions of a number of researchers at PSI were recognised in the scientific background to the 2023 Nobel Prize in Physics. These researchers include (L to R) Martin Huppert, Adrian Cavalieri and Stefan Neppl, all of whom are now working on the SwissFEL on advances that are enabling attosecond X-ray pulses. Here, they stand in the snow in the beautiful forest that surrounds SwissFEL.

Credit: Paul Scherrer Institute/Markus Fischer