BESSY II: Insight into ultrafast spin processes with femtoslicing

An international team has succeeded at BESSY II for the first time to elucidate how ultrafast spin-polarised current pulses can be characterised by measuring the ultrafast demagnetisation in a magnetic layer system within the first hundreds of femtoseconds. The findings are useful for the development of spintronic devices that enable faster and more energy-efficient information processing and storage. The collaboration involved teams from the University of Strasbourg, HZB, Uppsala University and several other universities.

Spintronic components are not based on moving charges, but on changes in the orientation of magnetic moments, such as electron spins. Spin-current-based devices can therefore operate extremely quickly, currently on time scales of up to one hundred picoseconds (one picosecond is 10-12 s). However, the microscopic processes themselves run much faster, in the range of a few hundred femtoseconds (1 fs = 10-15 s).

Magnetic layers form a spin valve

Now, an international team led by Prof. Christine Boeglin, University of Strasbourg, has been able to experimentally observe some of these particularly interesting dynamic processes in a magnetic layer system for the first time. They investigated a so-called spin valve consisting of alternating layers of platinum-cobalt and an iron-gadolinium alloy layer. In this system, interactions between excited (hot) electrons and magnetic layers are particularly strong. First author Deeksha Gupta and her colleagues conducted the experiments at the femtoslicing station at BESSY II together with the HZB team that is operating this worldwide unique infrastructure.

With a femtosecond infrared laser (IR), they generated hot electrons (HE) in a platinum (Pt) top layer. A thick copper layer (Cu, 60 nm) ensures that only HE pulses reach the Co/Pt layer at the front of the spin valve, which acted as a spin polariser, generating spin-polarised HE pulses (SPHE).

Read more on HZB website

Image: The scheme shows (from left to right): Hot electrons generated by a laser in platinum (light blue), the copper (yellow) is used to block the laser pulse so that only the hot electrons propagate and transport a spin current through the magnetic spin valve structure of cobalt platinum (blue-brown) and iron gadolinium (green).

Credit: D. Gupta /HZB

A piece of PSI history sets off on a long journey

Safely packed in a sturdy wooden crate, a high-tech component from PSI has begun its journey to Australia. The device was in use at PSI for more than ten years – now, with the commissioning of the Swiss X-ray free-electron laser SwissFEL, it has reached the end of its service life and will be given a new task at the Australian Synchrotron in Melbourne.

The device is carefully lifted by the indoor crane. The weight displayed on the crane’s external screen shoots up and down, eventually settling down at about 11.5 tonnes. The weight of this so-called insertion device is mainly due to its heavy steel frame. The magnets installed inside this generate attractive forces of several tonnes. The device must be able to withstand this enormous field strength. In particle accelerators, the periodic arrangement of the magnets is used to deflect electrons, thereby generating synchrotron radiation – a special type of X-rays.

Pioneering work at PSI

At PSI, the insertion device was used for a very special purpose, however. Following a lecture by an American colleague on the generation of ultra-short X-ray pulses, the two PSI physicists Gerhard Ingold and Thomas Schmidt realised that the conditions at the Swiss Light Source SLS were ideal for such a technique. The technology is called femtoslicing, and it can be used to observe extremely fast processes, such as chemical reactions.

“Immediately after the lecture was over, we did our first calculations. A few days later, the calculations turned into a project and three years later, under the leadership of Gerhard Ingold, we were finally able to produce hard X-rays in the femtosecond range for the first time in the world – a pulse of high-energy X-rays lasting 0.000 000 000 000 1 second,” as the head of the Insertion Device Group at PSI, Thomas Schmidt, recalls. Their approach was based on using the powerful magnetic field produced by this device as a modulator, so as to achieve resonance between the electrons and an external infrared laser, thereby transferring the pulse length of the latter to the X-rays. Since only a small fraction of the electrons are used in this process, namely those that overlap with the laser pulse, the technique is referred to as “slicing”.

The project resulted in numerous publications. Experiments were carried out on a range of different samples and new types of detectors were developed in order to process the extremely fast units of information. These findings were ultimately crucial to the development of free electron lasers, which are driven by linear accelerators and thus indirectly also the Swiss X-ray free-electron laser SwissFEL, where the first pilot experiments were carried out in 2017. However, this also heralded the end of the Femtoslicing Facility and thus of the insertion device in question. “SwissFEL allows us to generate much brighter and even shorter pulses of this kind of radiation than with the original facility. With this, extremely fast processes can be imaged at even higher resolutions,” says Thomas Schmidt.

Since then, the insertion device has been sitting in the hall of the SLS, unused.

Important manufacturer based in Siberia

Insertion devices are high-precision instruments, and demand for them is limited. Because of this, only a few manufacturers in the world are prepared to take on the complex task of building these devices in the first place. The world’s most important supplier of superconducting wigglers (a special type of insertion device) is based in Russia. However, due to the war and the global sanctions against Russia, many countries have also stopped importing these rare devices.

“Suddenly, there was a demand for retired wigglers in our European network for synchrotron radiation sources (LEAPS – League of European Accelerator-based Photon Sources),” explains Thomas Schmidt. “First, SOLARIS, the National Synchrotron Radiation Centre in Poland, inquired about a device that was no longer needed – we immediately agreed and sent them the plans. Unfortunately, our device was not compatible with their facility.” But just a short while later, the Australian Nuclear Science and Technology Organisation got in touch, also asking for a wiggler for their synchrotron in Melbourne. Again plans were sent – and this time everything fitted.

Read more on the PSI website

Image: Thomas Schmidt in the hall of the Swiss Light Source SLS. The insertion device weighing several tonnes can be seen suspended in the background, ready for transport. After being used for research at PSI more than ten years, this high-tech device will be given a new home at the Australian Synchrotron in Melbourne.

Credit: Paul Scherrer Institute/Mahir Dzambegovic