Superconductor exhibits “glassy” electronic phase

The study provides valuable insight into the nature of collective electron behaviors and how they relate to high-temperature superconductivity.

At extremely low temperatures, superconductors conduct electricity without resistance, a characteristic that’s already being used in cryogenically cooled power lines and quantum-computer prototypes. To apply this characteristic more widely, however, it’s necessary to raise the temperature at which materials become superconducting. Unfortunately, the exact mechanism by which this happens remains unclear.

Recently, scientists found that electrons in cuprate superconductors can self-organize into charge-density waves—periodic modulations in electron density that hinder the flow of electrons. As this effect is antagonistic to superconductivity, tremendous effort has been devoted to fully characterizing this charge-order phase and its interplay with high-temperature superconductivity.

>Read more on the Advanced Light Source at L. Berkeley Lab website

Image: At low doping levels, the charge correlations in the copper–oxide plane possess full rotational symmetry (Cinf) in reciprocal space (left), in marked contrast to all previous reports of bond-oriented charge order in cuprates. In real space (right), this corresponds to a “glassy” state with an apparent tendency to periodic ordering, but without any preference in orientation (scale bar ~5 unit cells).

Electric skyrmions charge ahead for next-generation data storage

Berkeley Lab-led research team makes a chiral skyrmion crystal with electric properties; puts new spin on future information storage applications.

When you toss a ball, what hand do you use? Left-handed people naturally throw with their left hand, and right-handed people with their right. This natural preference for one side versus the other is called handedness, and can be seen almost everywhere – from a glucose molecule whose atomic structure leans left, to a dog who shakes “hands” only with her right.

Handedness can be exhibited in chirality – where two objects, like a pair of gloves, can be mirror images of each other but cannot be superimposed on one another. Now a team of researchers led by Berkeley Lab has observed chirality for the first time in polar skyrmions – quasiparticles akin to tiny magnetic swirls – in a material with reversible electrical properties. The combination of polar skyrmions and these electrical properties could one day lead to applications such as more powerful data storage devices that continue to hold information – even after a device has been powered off. Their findings were reported this week in the journal Nature.

>Read more on the Advanced Light Source website

Image: Simulations of skyrmion bubbles and elongated skyrmions for the lead titanate/strontium titanate superlattice.
Credit: Berkeley Lab.

A designed material untangles long-standing puzzle

This approach could lead to new materials with emergent physics and unique electronic properties, supporting broader research efforts to revolutionize modern electronics.

When atoms or molecules assemble to form bulk matter, new properties (such as conductivity and ferromagnetism) that didn’t exist in the constituent parts can emerge from the whole. Similarly, stacking atomically thin layers into nanostructures (heterostructures) can give rise to a rich variety of emergent phases not found in bulk materials.

Materials that exhibit emergent phenomena (“quantum materials”) often feature multiple phases with simultaneous phase transitions. A great deal of effort is currently being expended to disentangle such transitions, to discover what drives them and to ultimately harness them in new materials with desired functionalities. Most of these efforts have relied on external perturbations (light, pressure, etc.) to decouple the transitions. In this work, researchers found a way to do this intrinsically, through layer-by-layer design of stacking sequences with mismatched periodicities.

>Read more on the Advanced Light Source website

Image: (a) Rare-earth (RE) nickelates (RENiO3) host multiple types of entangled orderings. This illustration depicts a magnetic ordering (spin directions indicated by yellow arrows) and a charge ordering (a checkerboard of two nickel oxidation states, indicated by sphere size and color) in bulk RENiO3 (RE and O atoms omitted for clarity). 
Please find the entire image here.