Ubiquitous formation of type-I and type-II bulk Dirac cones and topological surface states from a single orbital manifold in transition-metal dichalcogenides

Transition-metal dichalcogenides (TMDs) are renowned for their rich and varied properties. They range from metals and superconductorsto strongly spin-orbit-coupled semiconductors and charge-density-wave systems with their single-layer variants one of the most prominent current examples of two-dimensional materials beyond graphene.Their varied ground states largely depend on the transition metal d-electron-derived electronic states, on which the vast majority of attention has been concentrated to date.

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Image:Chalcogen-derived topological ladder in PdTe2.(a) Orbitally-resolved bulk electronic structure of PdTe2, indicating dominantly chalcogen-derived orbital character for the states in the vicinity of the Fermi level. (b) The measured out-of-plane dispersion together with the calculated band structure. Measured (c) and calculated (d) in-plane dispersion. (e,f) Spin-resolved energy distribution curves along the lines shown in (c).